I've been playing the OST obsessively for the last year of so. Songs like Battle of the Heroes, Palpatine's Teachings, Anakin's betrayal, are calming and paint a picture of Anakin's conflict much better than Hayden's wooden performance in ROTS. In terms of ROTS my favorite scene in the movie was Operation Knightfall, when a Young Vader goes in the Jed temple and lays waste to those sanctimonious fools.

The novelization to the film was farrr better than the film, from he description of Anakin's conflict to the extended description of how Mace was able to fight the Emperor while Tiin, Fisto, and Kolar got oneshot.