I'm starting to like Twilight Princess better than both of them. It mixes elements from Link to the Past and Ocarina of Time, and I'm liking the story so far as well. I'm about 35 hours into the game and I'd like to think I'm at least halfway finished.
Besides Zelda, I always thought that Goldeneye was one of the best Nintendo games ever. I used to play the hell out of that game when it first came out. I don't think I could go back and play it anymore though, as I simply refuse to play FPS's with a controller anymore. After playing Unreal Tournament with a mouse and keyboard nonstop for about a year, I could never go back to the controller. I can't play Halo on XBox either.