Not really. Maybe those are the only two scenes where they’re openly conflicting with each other, but in four out of five of the scenes they have together before they’re suddenly making out, Anakin’s being an asshole and pissing her off. I don’t know if that’s what you mean by a “facial feature thing”, but the emotions the actors are expressing convey the intended effect of the scene. Rewatch their first scene together in the movie. It cuts in reaction shots from Padmé, Captain Typho, and Jar Jar (!!) while Obi-Wan is spanking him to communicate to us that Anakin is making the whole room uncomfortable and being a huge dick. The scene uses Jar Jar to tell us to look down on Anakin’s behavior. What does she see in him?
Give me those scenes where he’s actively making her mad and she gets mad. What are they? Because I remember:
Scene where they meet, which isn’t him trying to make her mad, nor does she get mad.
Scene where he back talks Obi, which she doesn’t get mad at.
The you’re making me uncomfortable scene, which even in that scene is just Anakin and her talking until he gives her that look.
Then they exchange a little moment and joke about having R2.
They talk in transport about the Jedi rules. I think Anakin maybe is forward in this scene and she does have a tentative look, but no anger.
Then them walking through Naboo, a fairly amicable scene to me.
Then the scene where he gets mad about her saying he’s not a Jedi.
Then the sand and kiss scene.
Most of those moments between them aren’t angry at all, to me. That’s not even counting the scenes after that, where they talk near the waterfall or the scene and while they’re eating. Even the haunted by the kiss scene isn’t really about anger. Then there’s the tattooine stuff, which is all fairly amicable I think.